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Shown below is a rotationally resolved spectrum of the 0?0 vibrational band of a

ID: 2257119 • Letter: S

Question

Shown below is a rotationally resolved spectrum of the 0?0 vibrational band of an electronic transition in 89Y63Cu that was recorded in my laboratory. Measured wavenumbers of the observed rotational lines are given below the spectrum.

Line positions (cm?1):

11820.780

            11821.081

     11821.654

11822.700

11824.137

11820.811

            11821.152

     11821.786

11822.880

11824.375

11820.850

            11821.234

    11822.060

11823.071

11824.617

11820.896

            11821.323

    11822.204

11823.266

11824.873

11820.957

            11821.430

    11822.366

11823.472

11825.125

11821.011

            11821.537

   11822.527

11823.685

11825.398

11823.906

11825.674

(a). What branches are present in this spectrum? What are the first lines in these branches, labeled by the J?value of the lower state, J?? ?

(b). Does the rotational constant, B, increase or decrease when this electronic transition is excited?

(c). Does the bond length of the molecule, R, increase or decrease when this electronic transition is excited?

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(d). Compute the differences between successive lines in the list above. You should find that a regular pattern is observed, with the exception of one pair of lines that has a larger separation. After you locate this anomalously large separation, identify the observed lines using labels such as R(1), P(3), or Q(5). Make sure that the numbering of your lines is consistent with the branches you deduced in (a).

(e). One of the most useful methods of analyzing spectra makes use of what is rather obtusely called

11820.780

            11821.081

     11821.654

11822.700

11824.137

11820.811

            11821.152

     11821.786

11822.880

11824.375

11820.850

            11821.234

    11822.060

11823.071

11824.617

11820.896

            11821.323

    11822.204

11823.266

11824.873

11820.957

            11821.430

    11822.366

11823.472

11825.125

11821.011

            11821.537

   11822.527

11823.685

11825.398

11823.906

11825.674

Explanation / Answer

Shown below is a rotationally resolved spectrum of the 0?0 vibrational band of a

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